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Unravelling the optical responses of nanoplasmonic mirror-on-mirror metamaterials

机译:解开纳米等离子体反射镜超材料的光学响应

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摘要

Mirror-on-mirror platforms based on arrays of metallic nanoparticles, arranged top-down or self-assembled on a thin metallic film, have interesting optical properties. Interaction of localized surface-plasmons in nanoparticles with propagating surface-plasmons in the film underpins the exotic features of such platforms. Here, we present a comprehensive theoretical framework which emulates such a system using a five-layer-stack model and calculate its reflectance, transmittance, and absorbance spectra. The theory rests on dipolar quasi-static approximations incorporating image-forces and effective medium theory. Systematically tested against full-wave simulations, this simple approach proves to be adequate within its obvious applicability limits. It is used to study optical signals as a function of nanoparticle dimensions, interparticle separation, metal film thickness, the gap between the film and nanoparticles, and incident light characteristics. Several peculiar features are found, e.g., quenching of reflectivity in certain frequency domains or shift of the reflectivity spectra. Schemes are proposed to tailor those as functions of the mentioned parameters. Calculating the system's optical responses in seconds, as compared to much longer running simulations, this theory helps to momentarily unravel the role of each system parameter in light reflection, transmission, and absorption, facilitating thereby the design and optimisation of novel mirror-on-mirror systems.
机译:自上而下或自组装在金属薄膜上的基于金属纳米颗粒阵列的镜上镜平台具有令人感兴趣的光学特性。纳米粒子中的局部表面等离子体激元与薄膜中传播的表面等离子体激元的相互作用加强了此类平台的奇特特征。在这里,我们提供了一个综合的理论框架,该框架使用五层堆栈模型来模拟这样的系统,并计算其反射率,透射率和吸收光谱。该理论基于偶极准静态近似,该近似静态结合了像力和有效的介质理论。经过针对全波仿真的系统测试,这种简单的方法在其明显的适用范围内被证明是足够的。它用于研究光信号,这些信号是纳米颗粒尺寸,颗粒间分离,金属膜厚度,膜与纳米颗粒之间的间隙以及入射光特性的函数。发现了一些独特的特征,例如,在某些频域中反射率的猝灭或反射率谱的移动。提出了将这些参数定制为所提及参数的函数的方案。与更长的运行仿真相比,该算法可在几秒钟内计算出系统的光学响应,从而有助于暂时阐明每个系统参数在光反射,透射和吸收中的作用,从而有助于新型镜面镜的设计和优化。系统。

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